论文标题

形状波动和He $ _ {2}^{*}的光学过渡

Shape fluctuations and optical transition of He$_{2}^{*}$ excimer tracers in superfluid $^4$He

论文作者

Guo, Wei, Golov, Andrei I.

论文摘要

可稳定的He $ _ {2}^{*} $准分子分子已被用作超级流体$^4 $ He(He II)中正常成分的示踪剂颗粒,可以通过激光诱导的荧光成像。这些准分子分子在HE II中形成微小的气泡,可以在足够低的温度下与量化的涡流结合,从而可以直接可视化Inviscid超流体中的涡流动力学。但是,$ A^{3}σ^+_ {温度。在本文中,我们提出了一个气泡模型,用于评估HE II中准分子的表面波动本征模。 $ a^{3}σ^+_ {u} {\ rightArrow} c^{3}σ^+_ {g} $过渡是通过考虑零点和泡泡形状的零点的热波动来计算的。我们表明,随着温度从2〜K降至20 MK,峰吸收强度的增强了约5倍,并伴随着峰位置的蓝光速度约为2 nm。由于分子芯的旋转水平,可以解决双峰线轮廓。这个气泡模型还使我们能够评估He $ _ {2}^{*} $气泡的刚度,因此由于散射热声子而在He II中的扩散常数。我们的结果将有助于使用He $ _ {2}^{*} $ tracers进行成像量化涡流的未来实验。

Metastable He$_{2}^{*}$ excimer molecules have been utilized as tracer particles of the normal component in superfluid $^4$He (He II) which can be imaged via laser-induced fluorescence. These excimer molecules form tiny bubbles in He II and can bind to quantized vortices at sufficiently low temperatures, thereby allowing for direct visualization of vortex dynamics in an inviscid superfluid. However, the $a^{3}Σ^+_{u}$${\rightarrow}$$c^{3}Σ^+_{g}$ optical absorption line, which is responsible for the fluorescence imaging of the He$_{2}^{*}$ molecules, is controlled by fluctuations on the bubble shape, and its exact line profile is not known at low temperatures. In this paper, we present a bubble model for evaluating the surface fluctuation eigenmodes of the excimers in He II. The line profile of the $a^{3}Σ^+_{u}{\rightarrow}c^{3}Σ^+_{g}$ transition is calculated at different temperatures by considering both the zero-point and thermal fluctuations on the bubble shape. We show that, as the temperature drops from 2~K to 20 mK, the peak absorption strength is enhanced by a factor of about five, accompanying a blueshift of the peak location by about 2 nm. A double-peak line profile due to the rotational levels of the molecular core can be resolved. This bubble model also allows us to evaluate the stiffness of the He$_{2}^{*}$ bubbles and hence their diffusion constant in He II due to scattering off thermal phonons. Our results will aid the design of future experiments on imaging quantized vortices in He II using He$_{2}^{*}$ tracers.

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