论文标题
单层半导体螺旋钻检测器
Monolayer Semiconductor Auger Detector
论文作者
论文摘要
半导体中的螺旋体重组是一种多体现象,其中电子和孔的重组伴随着其他电荷载体的激发。它是非生育的,对光发射有害。激发载体的过量能量通常会迅速转化为热量,从而使螺旋过程很难直接探测。在这里,我们采用了一种技术,其中通过薄屏障可以从半导体中隧道隧道从半导体中隧道隧道隧道检测到,从而检测到螺旋杆兴奋的载体,从而产生电流。我们将垂直的范德华(VDW)异质结构用单层WSE2作为半导体,宽带隙六角形氮化硼(HBN)作为隧道屏障,以优先传输高能螺旋螺旋杆式载体,以优先传输到石墨电子上。当激发产生激发激发时,螺旋过程的明确特征是光电流的上升,以及由于电压与激子共振的变化而产生的负差异传统。我们检测到由中性和带电的激子都震撼的孔钻,并发现在较弱的激发下,螺旋螺旋散射令人惊讶地强。 VDW异质结构启用的低控制载体密度下的螺旋桨载体的选择性提取说明了可用于探测2D材料中松弛过程的技术的重要补充。
Auger recombination in semiconductors is a many-body phenomenon in which recombination of electrons and holes is accompanied by excitation of other charge carriers. Being nonradiative, it is detrimental to light emission. The excess energy of the excited carriers is normally rapidly converted to heat, making Auger processes difficult to probe directly. Here, we employ a technique in which the Auger-excited carriers are detected by their ability to tunnel out of the semiconductor through a thin barrier, generating a current. We employ vertical van der Waals (vdW) heterostructures with monolayer WSe2 as the semiconductor and the wide band gap hexagonal boron nitride (hBN) as the tunnel barrier to preferentially transmit high-energy Auger-excited carriers to a graphite electrode. The unambiguous signatures of Auger processes are a rise in the photocurrent when excitons are created by resonant excitation, and negative differential photoconductance resulting from the shifts of the exciton resonances with voltage. We detect holes Auger-excited by both neutral and charged excitons, and find that the Auger scattering is surprisingly strong under weak excitation. The selective extraction of Auger carriers at low, controlled carrier densities that is enabled by vdW heterostructures illustrates an important addition to the techniques available for probing relaxation processes in 2D materials.