论文标题

ENZ材料的快速和缓慢的非线性

Fast and slow nonlinearities in ENZ materials

论文作者

Khurgin, Jacob B., Clerici, Matteo, Kinsey, Nathaniel

论文摘要

具有增强的轻度相互作用功能的新型材料在实现非线性光学目标的崇高目标中起着至关重要的作用。最近,Epsilon-Near-Zero(ENZ)媒体已成为有前途的候选人,以增强包括折射率调制和谐波生成在内的几种非线性过程。在这里,我们分析了ENZ介质的光学非线性,以阐明与其他非线性媒体及其独特属性的共同点。我们专注于透明的导电氧化物(TCO)作为近红外(电信)频带中介电常数接近零的ENZ介质家族。我们研究了瞬时和延迟的非线性。通过从频带的非副代谢性中识别出它们的共同起源,我们表明它们的相对强度完全取决于能量和动量放松(或倾向)时间的比例。使用此框架,我们将ENZ材料与文献中已经进行了研究的许多有前途的非线性媒体进行了比较,并表明,ENZ材料在快速或缓慢的非线性中并没有从根本上超过传统材料的强度,但它们包含了关键的优势,例如理想的响应时间,例如理想的响应时间,固有的慢速度增强和宽带的宽带自然在compact式平台中用于使其成为超级适用于Ulterf的Phote for Ulters的范围。

Novel materials, with enhanced light-matter interaction capabilities, play an essential role in achieving the lofty goals of nonlinear optics. Recently, Epsilon-Near-Zero (ENZ) media have emerged as a promising candidate to enable the enhancement of several nonlinear processes including refractive index modulation and harmonic generation. Here, we analyze the optical nonlinearity of ENZ media to clarify the commonalities with other nonlinear media and its unique properties. We focus on transparent conducting oxides (TCOs) as the family of ENZ media with near zero permittivity in the near-infrared (telecom) band. We investigate the instantaneous and delayed nonlinearities. By identifying their common origin from the band nonparabolicity, we show that their relative strength is entirely determined by a ratio of the energy and momentum relaxation (or dephasing) times. Using this framework, we compare ENZ materials against the many promising nonlinear media that have been investigated in literature and show that while ENZ materials do not radically outpace the strength of traditional materials in either the fast or slow nonlinearity, they pack key advantages such as an ideal response time, intrinsic slow light enhancement, and broadband nature in a compact platform making them a valuable tool for ultrafast photonics applications for decades to come.

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