论文标题

通过与石墨烯中的声学,视听和表面极性声子耦合光激发电子的非弹性散射和冷却

Inelastic scattering and cooling of photoexcited electrons through coupling with acoustic, optic and surface polar optic phonons in graphene

论文作者

Khatoon, S. Arshia, Ansari, Meenhaz, Ashraf, S. S. Z., Obaidurrahman, M.

论文摘要

声学,光学和表面极性光学声子是三种重要的内在和外部语音模式,它们越来越多地在底物上填充石墨烯,温度升高。与电流方向的光激发热载体的耦合为电子 - 音波松弛提供了重要的途径。在本文中,我们从理论上研究了单层石墨烯中的三个语音模式在电子散射和冷却现象中的相对重要性,包括它们与超策略驱动的功率损失进行了比较,并获得了Boltzmann Transfort tommerity in the Electron-Phonon散射速率和冷却功率的能量依赖性的分析公式。所获得的分析溶液不仅与从较早报道的数值可牵引的积分形式获得的散射速率和冷却能力相关的结果,还使我们能够得出冷却时间和热电导的闭合形式公式。在所有三种模式的散射速率和冷却功率密度的估计中,还阐明了保障封锁的重要作用,阻止了阻止向填充能状态过渡的过渡。所获得的公式可以更好地了解热电子现象的动力学,从而明确观察了影响所研究运输量的不同变量的相互作用。该公式在数值优化方法中的性能优化的性能优化也可能有用,因为从这些公式中可以轻松地推论出一阶和二阶导数。

The acoustic, optic, and surface polar optic phonons are the three important intrinsic and extrinsic phononic modes that increasingly populate graphene on a substrate with rising temperatures; the coupling of which with photoexcited hot carriers in the equipartition regime provides significant pathways for electron-phonon relaxation. In this paper, we theoretically investigate the relative significance of the three phononic modes in electron scattering and cooling phenomena in single layer graphene, including their comparison with supercollision driven power loss, and obtain analytical formulae on the energy dependence of electron-phonon scattering rate and cooling power in the Boltzmann transport formalism. The obtained analytical solutions not only closely reproduce the results for scattering rate and cooling power, as that obtained from the earlier reported numerically tractable integral forms, but also enable us to derive closed-form formulae of the cooling time and thermal conductance. The important role of Pauli blocking that prevents transition to filled energy states has also been elucidated in the estimation of the scattering rate and cooling power density for all the three modes. The obtained formulae provide a better insight into the dynamics of hot electron phenomena giving an explicit view on the interplay of the different variables that affect the transport quantities under investigation. The formulae can also be potentially useful for performance optimization of transport quantities in numerical optimization methods since the first and second-order derivatives are easily deducible from these formulae.

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