论文标题

债券定向anapole订单中的旋转轨道耦合莫特绝缘子SR $ _2 $(ir $ _ {1-x} $ rh $ _x $)o $ _ {4} $

Bond Directional Anapole Order in a Spin-Orbit Coupled Mott Insulator Sr$_2$(Ir$_{1-x}$Rh$_x$)O$_{4}$

论文作者

Murayama, H., Ishida, K., Kurihara, R., Ono, T., Sato, Y., Kasahara, Y., Watanabe, H., Yanase, Y., Cao, G., Mizukami, Y., Shibauchi, T., Matsuda, Y., Kasahara, S.

论文摘要

一种抗反转和时间逆转对称性的Anapole状态,并保留了基础晶格的翻译对称性,引起了人们对新量子状态的极大兴趣,但仅报道了少数候选材料。最近,在旋转轨道耦合的莫特绝缘子\先生中,通过光学的第二次谐波生成测量值,已经在$t_Ω$上方提出了一个可能的隐藏订单阶段,其倒置对称性损坏。此外,偏光性中子衍射测量结果揭示了$t_Ω$以下的时间逆转对称性,随后的MUON自旋弛豫实验支持了$T_Ω$。但是,这个神秘阶段的本质在很大程度上仍然难以捉摸。在这里,我们通过具有异常高精度的磁性扭矩和具有弹性耐药性的列敏感性的平面磁各向异性的联合测量进行了研究。沿[110] IR-OIR键方向设置在$ \ simt_Ω$以下的两个平面内磁各向异性设置,为nematic相变的热力学证据提供了损坏的$ C_4 $旋转对称性。但是,与其他相关电子系统中报道的偶数列过渡相反,列敏感性对$t_Ω$没有不同的行为。这些结果为奇数顺序参数提供了大量证据,其旋转对称性在隐藏顺序状态下。我们讨论了一个隐藏的顺序,以一种阿波尔状态来讨论,在该状态下,每个IRO $ _6 $ _6 $ octhahedron of Ater Maghitality的两个循环诱发了极性旋转力矩。与先前建议的最简单的环电流模式相反,目前的结果与一个模式一致,在该模式中,单元内环环电流仅沿着IRO $ _4 $ Square中的对角线方向之一流动。

An anapole state that breaks inversion and time reversal symmetries with preserving translation symmetry of underlying lattice has aroused great interest as a new quantum state, but only a few candidate materials have been reported. Recently, in a spin-orbit coupled Mott insulator \SIR, the emergence of a possible hidden order phase with broken inversion symmetry has been suggested at $T_Ω$ above the Néel temperature by optical second harmonic generation measurements. Moreover, polarized neutron diffraction measurements revealed the broken time reversal symmetry below $T_Ω$, which was supported by subsequent muon spin relaxation experiments. However, the nature of this mysterious phase remains largely elusive. Here, we investigate the hidden order phase through the combined measurements of the in-plane magnetic anisotropy with exceptionally high-precision magnetic torque and the nematic susceptibility with elastoresistance. A distinct two-fold in-plane magnetic anisotropy along the [110] Ir-O-Ir bond direction sets in below $\sim T_Ω$, providing thermodynamic evidence for a nematic phase transition with broken $C_4$ rotational symmetry. However, in contrast to the even-parity nematic transition reported in other correlated electron systems, the nematic susceptibility exhibits no divergent behavior towards $T_Ω$. These results provide bulk evidence for an odd-parity order parameter with broken rotational symmetry in the hidden order state. We discuss the hidden order in terms of an anapole state, in which polar toroidal moment is induced by two current loops in each IrO$_6$ octahedron of opposite chirality. Contrary to the simplest loop-current pattern previously suggested, the present results are consistent with a pattern in which the intra-unit cell loop-current flows along only one of the diagonal directions in the IrO$_4$ square.

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