论文标题

SEESAW在COVID-19期间的排放减少与O $ _3 $增强的AOC之间的影响

The seesaw impacts between reduced emissions and enhanced AOC on O$_3$ during the COVID-19

论文作者

Zhu, Shengqiang, Poetzscher, James, Shen, Juanyong, Wang, Siyu, Wang, Peng, Zhang, Hongliang

论文摘要

由于2019年新型冠状病毒(Covid-19)大流行期间的锁定措施,经济活动和相关排放量大大下降。排放的减少创造了一个自然实验,以评估发射的前体控制政策对臭氧(O $ _3 $)污染的影响,这在过去十年中已成为中国的公众关注。在这项研究中,我们利用了全面的卫星,地面观测和面向来源的化学运输建模来调查中国Covid-19期间的O $ _3 $变化。在这里,我们发现o $ _3 $编队制度从VOC限制的制度转变为NOX有限的制度,这是由于COVID-19锁定期间的较低NOX。但是,中国平原(40%)和扬特河三角洲(35%)的o $ _3 $构造区域的这些变化主要归因于这些地区的增强大气氧化能力(AOC),这与以前的研究不同。我们建议未来的o $ _3 $控制政策应全面考虑O $ _3 $编队制度和AOC对O $ _3 $高程的协同影响。

Due to the lockdown measures during the 2019 novel coronavirus (COVID-19) pandemic, the economic activities and the associated emissions have significantly declined. This reduction in emissions has created a natural experiment to assess the impact of the emitted precursor control policy on ozone (O$_3$) pollution, which has become a public concern in China during the last decade. In this study, we utilized comprehensive satellite, ground-level observations, and source-oriented chemical transport modeling to investigate the O$_3$ variations during the COVID-19 in China. Here we found that the O$_3$ formation regime shifted from a VOC-limited regime to a NOx-limited regime due to the lower NOx during the COVID-19 lockdown. However, instead of these changes of the O$_3$ formation region, the significant elevated O$_3$ in the North China Plain (40%) and Yangtze River Delta (35%) were mainly attributed to the enhanced atmospheric oxidant capacity (AOC) in these regions, which was different from previous studies. We suggest that future O$_3$ control policies should comprehensively consider the synergistic effects of O$_3$ formation regime and AOC on the O$_3$ elevation.

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