论文标题

各向异性自旋分布和垂直磁各向异性在分层铁磁半导体(BA,K)(Zn,Mn)$ _ {2} $ as $ _ {2} $中

Anisotropic spin distribution and perpendicular magnetic anisotropy in the layered ferromagnetic semiconductor (Ba,K)(Zn,Mn)$_{2}$As$_{2}$

论文作者

Sakamoto, Shoya, Zhao, Guoqiang, Shibata, Goro, Deng, Zheng, Zhao, Kan, Wang, Xiancheng, Nonaka, Yosuke, Ikeda, Keisuke, Chi, Zhendong, Wan, Yuxuan, Suzuki, Masahiro, Koide, Tsuneharu, Tanaka, Arata, Maekawa, Sadamichi, Uemura, Yasutomo J., Jin, Changqing, Fujimori, Atsushi

论文摘要

新的铁磁半导体(BA,K)(Zn,Mn)$ _ {2} $作为$ _ {2} $的垂直磁各向异性是通过角度依赖的X射线磁性圆形二色dichroism测量结果研究的。通过将Stoner-Wohlfarth模型拟合到投影磁矩的磁场角依赖性,可以推断出具有0.85 T的各向异性场的大磁各向异性。横向XMCD光谱突出显示了Mn 3 $ d $电子的各向异性分布,其中$ d_ {xz} $和$ d_ {yz} $ orbitals比$ d_ {xy} $少了,因为从$ d_ {2d} $中散发出$ d_ {2d} $ splated of the e earlonged mnas $ snas $} $ _ {4建议磁各向异性起源于$ p $ - $ d_ {xz} $,$ d_ {yz} $杂交状态在费米级别上的变性,并且由于沿$ z $ z $方向对准旋转时旋转式偶联时产生的能量增益。

Perpendicular magnetic anisotropy of the new ferromagnetic semiconductor (Ba,K)(Zn,Mn)$_{2}$As$_{2}$ is studied by angle-dependent x-ray magnetic circular dichroism measurements. The large magnetic anisotropy with the anisotropy field of 0.85 T is deduced by fitting the Stoner-Wohlfarth model to the magnetic-field-angle dependence of the projected magnetic moment. Transverse XMCD spectra highlights the anisotropic distribution of Mn 3$d$ electrons, where the $d_{xz}$ and $d_{yz}$ orbitals are less populated than the $d_{xy}$ state because of the $D_{2d}$ splitting arising from the elongated MnAs$_{4}$ tetrahedra. It is suggested that the magnetic anisotropy originates from the degeneracy lifting of $p$-$d_{xz}$, $d_{yz}$ hybridized states at the Fermi level and resulting energy gain due to spin-orbit coupling when spins are aligned along the $z$ direction.

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