论文标题

不对称的Rydberg封锁巨大氧化物中的巨型激子

Asymmetric Rydberg blockade of giant excitons in Cuprous Oxide

论文作者

Heckötter, Julian, Walther, Valentin, Scheel, Stefan, Bayer, Manfred, Pohl, Thomas, Aßmann, Marc

论文摘要

通过高度激发的电子状态产生和控制强大的远程相互作用的能力已成为从原子和分子物理学[1,2]到量子光学[3,4]和技术[5-7]的许多领域突破的基础。 Rydberg激子提供了这种高度激发的状态的有希望的固态实现,在氧化混蛋半导体中确实已经观察到了纪录的轨道尺寸高达千分尺[8]。在这里,我们通过光学产生两个不同的rydberg激素态,证明了该材料中强激子相互作用的产生和控制。这使得两种彩色泵探针实验成为可能,可以详细探测相互作用。我们的实验揭示了强空间相关性的出现和一个州间的Rydberg阻滞,该封锁延伸到了非常大的几微米的距离上。产生的半导体激子的多体状态表现出普遍的特性,仅取决于相互作用的形状,并为其大大扩展范围和幂律特征产生明确的证据。

The ability to generate and control strong long-range interactions via highly excited electronic states has been the foundation for recent breakthroughs in a host of areas, from atomic and molecular physics [1, 2] to quantum optics [3, 4] and technology [5-7]. Rydberg excitons provide a promising solid-state realization of such highly excited states, for which record-breaking orbital sizes of up to a micrometer have indeed been observed in cuprous oxide semiconductors [8]. Here, we demonstrate the generation and control of strong exciton interactions in this material by optically producing two distinct quantum states of Rydberg excitons. This makes two-color pump-probe experiments possible that allow for a detailed probing of the interactions. Our experiments reveal the emergence of strong spatial correlations and an inter-state Rydberg blockade that extends over remarkably large distances of several micrometers. The generated many-body states of semiconductor excitons exhibit universal properties that only depend on the shape of the interaction potential and yield clear evidence for its vastly extended-range and power-law character.

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