论文标题
扫描探针显微镜的晶体学图像处理
Crystallographic image processing for scanning probe microscopy
论文作者
论文摘要
可以在晶体学上处理定期安排的对象的扫描探针显微镜(SPM)图像。结果信息可用于从SPM图像扭曲中删除,而SPM图像扭曲是由于不完美的成像过程所致。这些扭曲的综合作用导致点扩散功能,从而定量衡量显微镜在某些实验条件下的性能。根据高度对称的校准样品,可以提取并利用显微镜的点扩散功能来校正在基本相同的实验条件下记录的未知数的SPM图像。我们专注于我们方法的更多理论方面。钝性扫描隧道显微镜(STM)尖端由多个带有电子轨道尺寸的小型tips组成,可以根据二维周期性阵列的平面对称性的先验知识对称。通过在石墨上的常规氟化钴分子的STM图像的晶体学处理来说明这一点,并通过简单的模拟在概念上备份。
Scanning probe microscopy (SPM) images of regularly arranged spatially periodic objects can be processed crystallographically. The resulting information may be used to remove from the SPM image distortions that are due to a less than perfect imaging process. The combined effects of these distortions result in a point spread function that gives a quantitative measure of the performance of the microscope for a certain set of experimental conditions. On the basis of highly symmetric calibration samples, the point spread function of the microscope may be extracted and utilized for the correction of SPM images of unknowns that were recorded under essentially the same experimental conditions. We concentrate in this paper on more theoretical aspects of our method. A blunt scanning tunneling microscopy (STM) tip that consists of multiple mini-tips with electron orbital dimensions may be symmetrized on the basis of prior knowledge on the plane symmetry of a two-dimensional periodic array. This is illustrated with the crystallographic processing of a STM image of a regular array of fluorinated cobalt phthalocyanine molecules on graphite and backed up conceptually by simple simulations.