论文标题

Lacoo $ _ {3} $在超高磁场上的Spin-Triplet激子冷凝物的签名

Signature of spin-triplet exciton condensations in LaCoO$_{3}$ at ultrahigh magnetic fields up to 600 T

论文作者

Ikeda, Akihiko, Matsuda, Yasuhiro H., Sato, Keisuke, Ishii, Yuto, Sawabe, Hironobu, Nakamura, Daisuke, Takeyama, Shojiro, Nasu, Joji

论文摘要

自60年前预测以来,已经精力研究了电子孔对的Bose-Einstein凝结,即激子凝结。由于实验困难,在验证电荷中性和非磁性旋转弹性激子的凝结时仍缺乏无可辩驳的证据。尽管自旋超涡流和自旋分离效应将是可以观察到的,因此,自旋三刺激仪的凝结是一个有前途的前沿。在非常高的磁场下,规范的钴矿石lacoo $ _ {3} $是一个好的候选者,尚未得到验证。在这里,我们揭示了使用电磁通量压缩方法和最新的磁截面表生成的Lacoo $ _ {3} $的外来相图。我们发现了连续的磁曲线曲线和弯曲结构,这表明出现了两种不同的自旋三旋转激子冷凝物。通过构建现象学模型,我们表明激子的量子波动对于场诱导的连续过渡至关重要。三维且热平衡的钴矿石中的自旋三晶状体激子凝结为带有自旋 - 透明的旋转技术的新颖场所打开了一个新的场所,例如旋转的约瑟夫森连接。

Bose-Einstein condensation of electron-hole pairs, exciton condensation, has been effortfully investigated since predicted 60 years ago. Irrefutable evidence has still been lacking due to experimental difficulties in verifying the condensation of the charge neutral and non-magnetic spin-singlet excitons. Whilst, condensation of spin-triplet excitons is a promising frontier because spin supercurrent and spin-Seebeck effects will be observable. A canonical cobaltite LaCoO$_{3}$ under very high magnetic fields is a propitious candidate, yet to be verified. Here, we unveil the exotic phase diagram of LaCoO$_{3}$ up to 600 T generated using the electromagnetic flux compression method and the state-of-the-art magnetostriction gauge. We found the continuous magnetostriction curves and a bending structure, which suggest the emergence of two distinct spin-triplet exciton condensates. By constructing a phenomenological model, we showed that quantum fluctuations of excitons are crucial for the field-induced successive transitions. The spin-triplet exciton condensation in a cobaltite, which is three-dimensional and thermally equilibrated, opens up a novel venue for spintronics technologies with spin-supercurrent such as a spin Josephson junction.

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