论文标题
通过氮操纵绝缘ZRNX膜中超导穹顶的出现
Emergence of superconducting dome in insulating ZrNx films via nitrogen manipulation
论文作者
论文摘要
在基于Cu-,Fe-和Ni的化合物以外的其他材料中,重现密切相关的高过渡 - 温度(高-TC)超导体的电子相图是一项艰巨的任务。直到最近,一些材料系统通过乐队工程部分完成了这一目标。在这项工作中,我们将膜的生长,电荷传输,磁力测定法,Terahertz光谱,拉曼散射和扫描透射电子显微镜进行了研究,以研究超导性和ZRNX的正常状态,该相位图揭示了与高-TC超级导管的相似之处。值得注意的是,即使在Bardeen-Cooper-Schrieffer范式中可以表征ZRNX的超导性,并且可以通过调整N化学浓度在Fermi液体框架内理解其正常状态,但我们观察到在强烈的状态和正常状态的较高状态的近距离抗衡性的MIMICS MIMICS的近距离状态的超导圆顶的演变,我们会观察到超导圆顶的进化。
Reproducing the electronic phase diagram of strongly correlated high-transition-temperature (high-Tc) superconductors in materials other than Cu-, Fe-, and Ni-based compounds has been a challenging task. Only very recently, a few material systems have partially achieved this goal by band engineering. In this work, we combine film growth, charge transport, magnetometry, Terahertz Spectroscopy, Raman scattering, and Scanning Transmission Electron Microscopy to investigate superconductivity and the normal state of ZrNx, which reveals a phase diagram that bears extraordinary similarities to those of high-Tc superconductors. Remarkably, even though superconductivity of ZrNx can be characterized within the Bardeen-Cooper-Schrieffer paradigm and its normal state can be understood within the Fermi liquid framework, by tunning the N chemical concentration, we observe the evolution of a superconducting dome in the close vicinity of a strongly insulating state and a normal state resistivity mimics its counterpart of the high-Tc superconductors.