论文标题

挫折超导体re $ _2 $ hf中的时间反转对称性破裂

Time-reversal symmetry breaking in frustrated superconductor Re$_2$Hf

论文作者

Manda, Manasi, Kataria, Anshu, Patra, Chandan, Singh, D., Biswas, P. K., Hillier, A. D., Das, Tanmoy, Singh, R. P.

论文摘要

几何挫败感导致新颖的量子现象,例如三角形和卡戈梅晶格中的自旋液相。频段内和频段间的费米表面(FS)嵌套可以驱动独特的超导(SC)基地状态,分别具有$ d $ - 波和$ s^{\ pm} $配对对称性,根据SC差距在嵌套波形跨越嵌套波形的符号变化的标准。对于奇数的FSS,当多个带间嵌套具有可比的强度时,不同FS纸之间的标志反转标准会导致挫败感,从而促进新颖的SC顺序参数。在这里,我们报告了对FS嵌套挫败感引起的时间反转对称破坏配对状态的实验观察。此外,我们的电子特异性热和横向场$ $ $ $ SR实验表明配对对称性完全。第一原则电子结构计算揭示了具有相当带间嵌套强度的多个费米表面表。通过实现{\ it ab-initio}频带结构,我们计算自旋 - 触发介导的SC配对对称性,揭示了$ s+是'$ - 配对状态 - 与实验观察一致。我们的调查表明了一种新型的SC状态,该状态为应用和基础研究提供了假定的设置。

Geometrical frustration leads to novel quantum phenomena such as the spin-liquid phase in triangular and Kagomé lattices. Intra-band and inter-band Fermi surface (FS) nesting can drive unique superconducting (SC) ground states with $d$-wave and $s^{\pm}$ pairing symmetries, respectively, according to the criterion that the SC gap changes sign across the nesting wavevector. For an odd number of FSs, when multiple inter-band nesting is of comparable strength, the sign-reversal criterion between different FS sheets can leads to frustration, which promotes novel SC order parameters. Here we report the experimental observation of a time-reversal symmetry breaking pairing state in Re$_2$Hf resulting from FS nesting frustration. Furthermore, our electronic specific heat and transverse-field $μ$SR experiments suggest a fully gaped pairing symmetry. The first-principle electronic structure calculation reveals multiple Fermi surface sheets with comparable inter-band nesting strength. Implementing the {\it ab-initio} band structure, we compute spin-fluctuation mediated SC pairing symmetry which reveals a $s+is'$-pairing state - consistent with experimental observations. Our investigation demonstrates a novel SC state which provides a putative setting for both applied and fundamental study.

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