论文标题
测量微型和纳米结构表面的复杂性
Measuring the complexity of micro and nanostructured surfaces
论文作者
论文摘要
纳米结构表面通常表现出复杂的形态,这些形态无法用欧几里得几何形状描述。同时,它们并不构成完全由简单的随机性和概率理论来表征的完全随机噪声场。在大多数情况下,纳米形态由复杂的秩序和随机性混合物组成,如果人们旨在控制其制造和特性,则应定量描述。在这项工作中,受复杂性理论的最新发展的启发,我们提出了一种基于与表面平均对称性偏差的纳米形态复杂性的方法。我们使用一系列合成表面介绍了其计算和验证其性能的方法,其中提议的复杂性度量在完全有序的和完全随机的病例之间以最异构的形态获得了最大值。此外,我们测量了实验微观和纳米结构表面(聚合物和金属)的复杂性,并证明了所提出的方法在量化加工条件对其形态的影响时的有用性。最后,我们暗示了复杂度度量与表面的功能特性之间的关系。
Nanostructured surfaces usually exhibit complicated morphologies that cannot be described in terms of Euclidean geometry. Simultaneously, they do not constitute fully random noise fields to be characterized by simple stochastics and probability theory. In most cases, nanomorphologies consist of complicated mixtures of order and randomness, which should be described quantitatively if one aims to control their fabrication and properties. In this work, inspired by recent developments in complexity theory, we propose a method to measure nanomorphology complexity that is based on the deviation from the average symmetry of surfaces. We present the methodology for its calculation and the validation of its performance, using a series of synthetic surfaces where the proposed complexity measure obtains a maximum value at the most heterogeneous morphologies between the fully ordered and fully random cases. Additionally, we measure the complexity of experimental micro and nanostructured surfaces (polymeric and metallic), and demonstrate the usefulness of the proposed method in quantifying the impact of processing conditions on their morphologies. Finally, we hint on the relationship between the complexity measure and the functional properties of surfaces.