论文标题
混合2D-QD MOS2 PBSE量子点宽带光电探测器具有高敏性和2.5μm的室温操作
Hybrid 2D-QD MoS2 PbSe Quantum Dot Broadband Photodetectors with High-Sensitivity and Room-Temperature Operation at 2.5 μm
论文作者
论文摘要
宽带红外光电探测器在包括安全性,气体传感,生物成像,食品质量的光谱和回收利用的各种应用中非常重要,仅举几例。但是,这些应用程序目前可以由昂贵的外延型光电探测器提供服务,从而限制了它们的市场潜力和社会影响。在混合布局中使用胶体量子点(CQD)和2D材料是设计低成本CMOS兼容的红外光探测器的有吸引力的替代品。然而,这些常规杂种探测器的光谱灵敏度局限于2.1 um。在本文中,我们提出了一个杂种结构,其中包括带有PBSE CQD的MOS2,以将其灵敏度进一步扩展到中波红外,最高为3 um。我们的室温响应性达到137.6 A/W,由于在MOS2和PBSE的界面处高效的光激发载体分离,探测器在2.55 um处于2.55 um,并与氧化物涂层结合使用以减少黑电流;基于PBSE的混合设备的最高值。这些发现强烈支持成功制造混合设备,这些设备可能为具有成本效益,高性能,下一代,新型光电遗传学的途径铺平了途径。
Broadband infrared photodetectors have profound importance in diverse applications including security, gas sensing, bioimaging, spectroscopy for food quality, and recycling, just to name a few. Yet, these applications can currently be served by expensive epitaxially grown photodetectors, limiting their market potential and social impact. The use of colloidal quantum dots (CQDs) and 2D-materials in a hybrid layout is an attractive alternative to design low-cost CMOS-compatible infrared photodetectors. However, the spectral sensitivity of these conventional hybrid detectors has been restricted to 2.1 um. Herein, we present a hybrid structure comprising MoS2 with PbSe CQDs to extend their sensitivity further towards the mid-wave infrared, up to 3 um. We achieve room temperature responsivity of 137.6 A/W and a detectivity of 7.7 10^10 Jones at 2.55 um owing to highly efficient photoexcited carrier separation at the interface of MoS2 and PbSe in combination with an oxide-coating to reduce dark current; the highest value yet for a PbSe based hybrid device. These findings strongly support the successful fabrication of hybrid devices which may pave the pathway for cost-effective, high performance, next-generation, novel photodetectors.