论文标题
磁性kagome超导体ceru $ _2 $
Magnetic Kagome Superconductor CeRu$_2$
论文作者
论文摘要
带有Kagome晶格的材料为寻找新的电子相位提供了一个平台,并研究了相关与拓扑之间的相互作用。最近,各种探针表明,kagome晶格可以用相互缠绕的顺序构成各种量子相,包括电荷密度波状态,键密度波态,手性电荷顺序,以及很少有超导性。但是,关于kagome材料中超导性和磁性共存的报道仍然难以捉摸。在这里,我们通过Ru Atoms形成的Kagome网络重新访问磁性超导体CERU $ _2 $。我们的第一原理计算显示,在费米表面附近的kagome平面带,表明扁平磁力磁性。在环境压力下,CERU $ _2 $表现出超导过渡温度($ t _ {\ text {c}} $),最大〜6 k,磁性顺序在〜40 k处。值得注意的是,可以通过调整RU的量来调节超导性和相关行为。我们通过磁性,电阻率和结构测量在高达〜168 GPA的压力下进行了对CERU $ _2 $中超导和磁性的系统研究。一个不寻常的相图表明,已经构建了化合物的超导顺序参数之间有趣的相互作用。在〜28 gpa的压力上观察到$ t _ {\ text {c}} $复苏,并伴随着次级超导过渡的突然出现。我们的实验已经确定了由高压驱动的诱人的相变,并表明CERU $ _2 $中的超导性和磁性很强。
Materials with a kagome lattice provide a platform for searching for new electronic phases and investigating the interplay between correlation and topology. Various probes have recently shown that the kagome lattice can host diverse quantum phases with intertwined orders, including charge density wave states, bond density wave states, chiral charge order, and, rarely, superconductivity. However, reports of the coexistence of superconductivity and magnetic order in kagome materials remain elusive. Here we revisit a magnetic superconductor CeRu$_2$ with a kagome network formed by Ru atoms. Our first-principles calculations revealed a kagome flat band near the Fermi surface, indicative of flat-band magnetism. At ambient pressure, CeRu$_2$ exhibits a superconducting transition temperature ($T_{\text{c}}$) up to ~ 6 K and a magnetic order at ~ 40 K. Notably, superconductivity and related behavior can be tuned by adjusting the amount of Ru. We conducted a systematic investigation of the superconductivity and magnetic order in CeRu$_2$ via magnetic, resistivity, and structural measurements under pressure up to ~ 168 GPa. An unusual phase diagram that suggests an intriguing interplay between the compound's superconducting order parameters has been constructed. A $T_{\text{c}}$ resurgence was observed above pressure of ~ 28 GPa, accompanied by the sudden appearance of a secondary superconducting transition. Our experiments have identified tantalizing phase transitions driven by high pressure and suggest that the superconductivity and magnetism in CeRu$_2$ are strongly intertwined.