论文标题

时间相关滤波显示强场电离中的两路电子量子干扰

Time Correlation Filtering Reveals Two-Path Electron Quantum Interference in Strong-Field Ionization

论文作者

Werby, Nicholas, Maxwell, Andrew S., Forbes, Ruaridh, Faria, Carla Figueira de Morisson, Bucksbaum, Philip H.

论文摘要

强场隧道电离中的Attsond动力学在光电子动量分布(PMD)中以复杂的全息图(PMD)编码。这些模式显示了两个或多个超量的量子电子轨迹之间的干扰,这些量子轨迹由它们的电离时间和随后在激光场中的进化来定义。我们通过对测得的动量光谱进行差异傅立叶分析来确定干扰电子轨道对之间的电离时间分离。我们确定由轨迹对形成的电子全息图,其电离时间的分离小于一个四分之一周期,在四分之一周期至一半循环之间,在半个周期至四分之三的循环之间,而整个周期则分开。我们将实验结果与库仑量子轨道强场近似(CQSFA)的预测进行了比较,并取得了巨大的成功。我们还会过滤CQSFA轨迹计算,以证明该技术在光谱上具有已知时间相关的有效性。作为一般分析技术,可以将过滤器应用于所有能量和角度分辨的数据集,以恢复干扰电子途径之间的时间相关性,从而提供了一个重要的工具来分析任何强场电离光谱。

Attosecond dynamics in strong-field tunnel ionization are encoded in intricate holographic patterns in the photoelectron momentum distributions (PMDs). These patterns show the interference between two or more superposed quantum electron trajectories, which are defined by their ionization times and subsequent evolution in the laser field. We determine the ionization time separation between interfering pairs of electron orbits by performing a differential Fourier analysis on the measured momentum spectrum. We identify electron holograms formed by trajectory pairs whose ionization times are separated by less than a single quarter cycle, between a quarter cycle and half cycle, between a half cycle and three fourths of a cycle, and a full cycle apart. We compare our experimental results to the predictions of the Coulomb quantum orbit strong-field approximation (CQSFA), with significant success. We also time-filter the CQSFA trajectory calculations to demonstrate the validity of the technique on spectra with known time correlations. As a general analysis technique, the filter can be applied to all energy- and angularly-resolved datasets to recover time correlations between interfering electron pathways, providing an important tool to analyze any strong-field ionization spectra.

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