论文标题

钻石砧室内的第二个谐波交流量热法

Second harmonic AC calorimetry technique within a diamond anvil cell

论文作者

Dasenbrock-Gammon, Nathan, McBride, Raymond, Yoo, Gyeongjae, Dissanayake, Sachith, Dias, Ranga

论文摘要

在高压下调整物质的能量密度会产生异国情调的和通常是前所未有的特性,例如结构过渡,绝缘剂 - 金属转变,价波动,拓扑顺序以及超导性的出现。长期以来,对特定热量的研究已被用来表征这些类型的过渡,但事实证明,它们在钻石砧细胞(DAC)环境中的应用已具有挑战性。在测量DAC内的特定热量方面的工作有限,部分原因是实验设置困难。为此,我们开发了一种新的方法来测量DAC内的特定热量,该方法与DAC设计无关,因此很容易与已经执行高压电阻测量的任何DAC兼容。作为概念验证,进行了MGB2超导体的特定热测量值,显示在过渡温度(TC)处明显的异常,这表明散装超导性。该技术允许在压力更高的情况下进行比以前更高的热量测量。

Tuning the energy density of matter at high pressures gives rise to exotic and often unprecedented properties, e.g., structural transitions, insulator-metal transitions, valence fluctuations, topological order, and the emergence of superconductivity. The study of specific heat has long been used to characterize these kinds of transitions, but their application to the diamond anvil cell (DAC) environment has proved challenging. Limited work has been done on the measurement of specific heat within DACs, in part due to the difficult experimental setup. To this end we have developed a novel method for the measurement of specific heat within a DAC that is independent of the DAC design and therefore readily compatible with any DACs already performing high pressure resistance measurements. As a proof-of-concept, specific heat measurements of the MgB2 superconductor were performed, showing a clear anomaly at the transition temperature (Tc), indicative of bulk superconductivity. This technique allows for specific heat measurements at higher pressure than previously possible.

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