论文标题

低损坏等离子体纳米腔启用的六角硼氮化硼中自旋缺陷的发射大大增强

Greatly Enhanced Emission from Spin Defects in Hexagonal Boron Nitride Enabled by a Low-Loss Plasmonic Nano-Cavity

论文作者

Xu, Xiaohui, Solanki, Abhishek. B., Sychev, Demid, Gao, Xingyu, Peana, Samuel, Baburin, Aleksandr S., Pagadala, Karthik, Martin, Zachariah O., Chowdhury, Sarah N., Chen, Yong P., Rodionov, Ilya A., Kildishev, Alexander V., Li, Tongcang, Upadhyaya, Pramey, Boltasseva, Alexandra, Shalaev, Vladimir M.

论文摘要

众所周知,二维六角硼(HBN)具有各种量子发射器,具有适用于广泛量子光子应用的性能。其中,由于其在量子传感中的潜在用途,最近出现了带有可寻址自旋状态的带负电荷的硼空位(VB)缺陷。与散装晶体中的自旋缺陷相比,当将其放置在距HBN表面的纳米尺寸距离处时,VB可以保留其自旋相干性能,从而使纳米尺度量子量子传感。另一方面,VB的低量子效率阻碍了其在实际应用中的使用。几项研究报告说,使用等离子体效应提高了VB缺陷的总量子效率。但是,迄今为止报告的最多17次的总体增强功能相对较小。在这项研究中,我们探索并证明了通过超低纳米点天线(NPA)结构的Vb增强的较高的发射增强。对于NPA耦合的VB缺陷,观察到高达250次的总强度增强。由于激光斑点超过了发生增强的NPA面积,因此NPA提供的实际增强率为约1685次,这比先前报道的结果显着增加。重要的是,在这种异常强大的增强下,保留了光学检测到的磁共振(ODMR)对比度。我们的结果不仅建立了NPA耦合的VB缺陷,因为在弱激光功率下运行的高分辨率磁场传感器,而且还为获得单个VB缺陷提供了有希望的方法。

Two-dimensional hexagonal boron nitride (hBN) has been known to host a variety of quantum emitters with properties suitable for a broad range of quantum photonic applications. Among them, the negatively charged boron vacancy (VB-) defect with optically addressable spin states has emerged recently due to its potential use in quantum sensing. Compared to spin defects in bulk crystals, VB- preserves its spin coherence properties when placed at nanometer-scale distances from the hBN surface, enabling nanometer-scale quantum sensing. On the other hand, the low quantum efficiency of VB- has hindered its use in practical applications. Several studies have reported improving the overall quantum efficiency of VB- defects using plasmonic effects; however, the overall enhancements of up to 17 times reported to date are relatively modest. In this study, we explore and demonstrate much higher emission enhancements of VB- with ultralow-loss nano-patch antenna (NPA) structures. An overall intensity enhancement of up to 250 times is observed for NPA-coupled VB- defects. Since the laser spot exceeds the area of the NPA, where the enhancement occurs, the actual enhancement provided by the NPA is calculated to be ~1685 times, representing a significant increase over the previously reported results. Importantly, the optically detected magnetic resonance (ODMR) contrast is preserved at such exceptionally strong enhancement. Our results not only establish NPA-coupled VB- defects as high-resolution magnetic field sensors operating at weak laser powers, but also provide a promising approach to obtaining single VB- defects.

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