论文标题

由于域成核的逆转而导致的福克图图特征

FORC Diagram Features of Co Particles due to Reversal by Domain Nucleation

论文作者

Breth, Leoni, Fischbacher, Johann, Kovacs, Alexander, Özelt, Harald, Schrefl, Thomas, Brückl, Hubert, Czettl, Christoph, Kührer, Saskia, Pachlhofer, Julia, Schwarz, Maria

论文摘要

一阶反转曲线(FORC)图是地球物理和材料科学中的流行工具,用于表征自然和合成起源的磁颗粒。但是,关于福克图图中某些特征的起源的严格解释仍然存在很多争议。在这项研究中,我们分析了通过尺寸为50、100和150 nm和单轴磁晶的CO立方计算的FORCS。对于较大的立方体,我们观察到稳定的两域状态的形成。反向域及其随后的an灭的成核清楚地视为福克图中的单独峰。它们沿福克斯图中的坐标轴散布,这与Preisach Hysteron的偏置场$ H_U $相关。根据我们的发现,我们指出,沿$ H_U $轴扩散的福克图峰可以起源于由单个粒子中域的成核驱动的逐步磁化逆转逆转。这意味着,除了一组粒子之间的众所周知的磁相互作用外,我们已经确定了另一种机制,该粒子会导致沿$ H_U $轴扩展的FORC图中的特征。我们的研究表明,如果应将福克斯用作评估含有磁性材料样品的微观结构的定量工具,则需要更多来自其他方法的信息来确定在福克图图中生产某些“指纹”的正确物理机制。

First Order Reversal Curve (FORC) diagrams are a popular tool in geophysics and materials science for the characterization of magnetic particles of natural and synthetic origin. However, there is still a lot of controversy about the rigorous interpretation of the origin of certain features in a FORC diagram. In this study, we analyze FORCs computed by micromagnetic simulations of Co cubes with dimensions of 50, 100 and 150 nm and uniaxial magnetocrystalline anisotropy. For the larger cubes we observe the formation of a stable two-domain state. The nucleation of a reversed domain and its subsequent annihilation are clearly visible as separate peaks in the FORC diagram. They spread out along the coordinate axis in the FORC diagram, which is associated with the bias field $H_U$ of a Preisach hysteron. Based on our findings, we state that a FORC diagram peak spreading along the $H_U$ axis can have its origin in the step-wise magnetization reversal driven by nucleation of domains in a single particle. This means that we have identified another mechanism apart from the well-known magnetostatic interaction between a set of particles that leads to features in the FORC diagram extending along the $H_U$-axis. Our study demonstrates that if FORCs shall be used as a quantitative tool to assess the microstructure of samples containing magnetic material, more information from other methods will be required to identify the correct physical mechanism by which a certain "fingerprint" in a FORC diagram is produced.

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