论文标题

中心对称skyrmion宿主材料GD2PDSI3上的偏振中子散射研究

Polarized neutron scattering study on the centrosymmetric skyrmion host material Gd2PdSi3

论文作者

Ju, Jiwon, Saito, Hiraku, Kurumaji, Takashi, Hirschberger, Max, Kikkawa, Akiko, Taguchi, Yasujiro, Arima, Taka-hisa, Tokura, Yoshinori, Nakajima, Taro

论文摘要

我们已经通过具有富含同位素160GD的单晶的零场散射在零场附近的偏振中子散射中研究了中心对称性skyrmion材料GD2PDSI3的磁结构。在先前的研究中,通过谐振X射线散射测量结果研究了低温下GD2PDSI3中的磁结构[T. Kurumaji等。科学365,914(2019)]。目前的极化中子结果证实,零场中的磁结构具有椭圆螺钉型磁调制,其传播向量为(q,0,0),Q〜0.14及其等效物。随着温度的升高,系统会经历磁相跃迁,同时保持(Q,0,0)的不相称的Q-vector。我们发现,热诱导的相具有正弦磁调节,磁矩垂直于C轴和Q矢量。我们还通过极化中子研究了基态下的自旋螺旋度自由度,表明该系统包含左手和右手螺钉型的相等分数,如中心对称晶体结构所预期的。

We have investigated magnetic structures of the centrosymmetrric skyrmion material Gd2PdSi3 by means of polarized neutron scattering near zero field with an isotope-160Gd-enriched single crystal. In a previous study, magnetic structures in Gd2PdSi3 at low temperatures were studied by resonant X-ray scattering measurements [T. Kurumaji et al. Science 365, 914 (2019)]. The present polarized neutron results confirm that the magnetic structure in zero field has elliptic screw-type magnetic modulation with a propagation vector of (q, 0, 0) with q ~ 0.14 and its equivalents. As the temperature increases, the system undergoes a magnetic phase transition while keeping the incommensurate q-vector of (q,0,0). We found that the thermally-induced phase has sinusoidal magnetic modulations with magnetic moments perpendicular both to the c axis and to the q-vector. We also investigate the spin-helicity degree of freedom in the ground state by polarized neutrons, revealing that the system contains equal fractions of the left-handed and right-handed screw-type orders as expected from the centrosymmetric crystal structure.

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