论文标题

FERHCRSI:一种具有室温自旋阀行为的新自旋半学

FeRhCrSi: A new spin semimetal with room temperature spin-valve behavior

论文作者

Venkateswara, Y., Nag, Jadupati, Samatham, S. Shanmukharao, Patel, Akhilesh Kumar, Babu, P. D., Varma, Manoj Raama, Nayak, Jayita, Suresh, K. G., Alam, Aftab

论文摘要

旋转半法是最近发现的新型自旋材料类,它们在一个自旋通道中显示带隙,而另一个自旋材料则具有半金属特征,因此可以进行可调的自旋传输。在这里,我们介绍了Ferhcrsi中自旋半金属行为的实验验证,Ferhcrsi是一种饱和矩2 $μ_b$和居里温度$> $ 400 k的季节旋转合金。它在L2 $ _1 $结构中结晶为50 $ \%$ \%$ \%$ \%的fe和RH之间。低于300 K,它显示了弱温度系数的弱温度依赖性电阻率,表明正常的半准或旋转半明确行为。异常的磁化磁性数据揭示了不对称部分的主要贡献,这是自旋阀自然的明确特征,即使在室温下也可以保留。 \ textColor {black} {磁性抗性的不对称部分随温度的升高显示出异常增加。}霍尔测量结果证实了来自固有浆果曲率的电导率的异常性质,孔是多数载体。 Ab-Initio模拟证实了独特的远程铁磁命令是基态,这解释了意外的低饱和力矩背后的起源。通过实验观察到的,铁磁性无序结构证实了FERHCRSI的自旋半金属特征。

Spin semimetals are a recently discovered new class of spintronic materials, which exhibit a band gap in one spin channel while a semimetallic feature in the other and thus allows for tunable spin transport. Here, we present experimental verification of spin semimetallic behavior in FeRhCrSi, a quaternary Heusler alloy with saturation moment 2 $μ_B$ and Curie temperature $>$ 400 K. It crystallises in the L2$_1$ structure with 50$\%$ antisite disorder between Fe and Rh. Below 300 K, it shows a weakly temperature dependent electrical resistivity with negative temperature coefficient, indicating the normal semimetal or spin semimetal behavior. Anomalous magnetoresistance data reveals dominant contribution from asymmetric part, a clear signature of spin-valve nature, which is retained even at room temperature. \textcolor{black}{The asymmetric part of magneto-resistance shows an unusual increase with increasing temperature.} Hall measurements confirm the anomalous nature of conductivity originating from the intrinsic Berry curvature, with holes being the majority carriers. Ab-initio simulation confirms a unique long-range ferrimagnetic ordering to be the ground state, explaining the origin behind the unexpected low saturation moment. The ferrimagnetic disordered structure confirms the spin semimetallic feature of FeRhCrSi, as observed experimentally.

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