论文标题
无序的超均匀固态材料
Disordered Hyperuniform Solid State Materials
论文作者
论文摘要
最近发现的凝结物质的异国情调状态最近被发现。 DHU系统与液体或眼镜相似,因为它们在统计学上是各向同性的,并且缺乏常规的远距离翻译和定向顺序。另一方面,它们完全抑制了像晶体这样的归一化无限波长密度波动,并且从这个意义上讲,它们具有隐藏的远距离顺序。最近,在固态材料中有几个令人兴奋的过度均匀性发现,包括无定形碳纳米管,无定形二氧化硅,无定形石墨烯,缺陷的过渡金属二分法,缺陷,五边形2D材料和中等/高输入合金。已经发现,这些材料的DHU状态通常比其他疾病模型具有明显低的能量,并且可能导致独特的电子和热传输特性,这是由与晶体鉴定的机制不同的机制所产生的。例如,DHU状态可以增强2D无定形二氧化硅的电子传输。 DHU培养基/高渗透合金实现了Vegard的定律,并在低温下具有增强的电子带隙和热传输。这些独特的特性为光电和热电学提供了许多有希望的潜在设备应用。在这里,我们对固态材料中超均匀性的这些重要新事物进行了重点评论,采用了应用和``材料''的观点,可以补充现有的关于物理系统和光子材料中超均匀性的评论。还提供了未来的方向和前景,重点是设计和发现用于量子信息科学和工程的DHU量子材料。
Disordered hyperuniform (DHU) states are recently discovered exotic states of condensed matter. DHU systems are similar to liquids or glasses in that they are statistically isotropic and lack conventional long-range translational and orientational order. On the other hand, they completely suppress normalized infinite-wavelength density fluctuations like crystals, and in this sense possess a hidden long-range order. Very recently, there are several exciting discoveries of disordered hyperuniformity in solid-state materials, including amorphous carbon nanotubes, amorphous 2D silica, amorphous graphene, defected transition metal dichalcogenides, defected pentagonal 2D materials, and medium/high-entropy alloys. It has been found the DHU states of these materials often possess a significantly lower energy than other disorder models, and can lead to unique electronic and thermal transport properties, which resulted from mechanisms distinct from those identified for their crystalline counterparts. For example, DHU states can enhance electronic transport in 2D amorphous silica; DHU medium/high-entropy alloys realize the Vegard's law, and possess enhanced electronic band gaps and thermal transport at low temperatures. These unique properties open up many promising potential device applications in optoelectronics and thermoelectrics. Here, we provide a focused review on these important new developments of hyperuniformity in solid-state materials, taking an applied and ``materials'' perspective, which complements the existing reviews on hyperuniformity in physical systems and photonic materials. Future directions and outlook are also provided, with a focus on the design and discovery of DHU quantum materials for quantum information science and engineering.