论文标题

强场电离和AC-Stark在OC中移动了Rydberg国家

Strong-field ionization and AC-Stark shifted Rydberg states in OCS

论文作者

Abu-samha, Mahmoud, Madsen, Lars Bojer

论文摘要

我们介绍了强度依赖性阈值离子化(ATI)光谱的理论结果,该光谱是由强烈的飞秒激光脉冲探测的,波长为800 nm和400 nm。使用单活动电子近似中的时间依赖性Schrooodinger方程进行计算,并包括多电体极化效应。结果与实验数据有定性一致[Yu等,J。Phys。 B:at。摩尔。选择。物理。 50,235602(2017)]。特别是,该理论捕获了ATI光谱中通过高度激发的Rydberg状态对应于通过高度激发的Rydberg状态的共振多光子离子化的特征。

We present theoretical results for intensity-dependent above-threshold ionization (ATI) spectra from oriented OCS molecules probed by intense femtosecond laser pulses with wavelengths of 800 and 400 nm. The calculations were performed using the time-dependent Schroodinger equation within the single-active-electron approximation and including multielectron polarization effects. The results are in qualitative agreement with experimental data [Yu et al., J. Phys. B: At. Mol. Opt. Phys. 50, 235602 (2017)]. In particular, characteristic features in the ATI spectra which correspond to resonant multiphoton ionization via highly-excited Rydberg states are captured by the theory.

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