论文标题
蒙特卡洛模拟金纳米颗粒的辐射效应的实验基准数据。第二部分:比较金纳米丝的测量和模拟电子光谱
Experimental benchmark data for Monte Carlo simulated radiation effects of gold nanoparticles. Part II: Comparison of measured and simulated electron spectra from gold nanofoils
论文作者
论文摘要
光子相互作用后的薄金箔的电子发射光谱在50 eV和9500 eV之间测量,以提供蒙特卡罗辐射传输模拟的参考数据。在Desy(德国汉堡)的Petra III高毛线束P22上使用HAXPES光谱仪进行实验,以在每个金色L-Edges(即11.9 Kev,12.0 Kev,12.0 Kev,12.0 Kev,13.7 Kev,13.7 Kev,13.8 Kev,13.8 Kev,14.3 Kev,14.3 kev)和14.4.4.4 kev和14.4 kev中,略高于和上方。分析数据以获得每个入射光子通量发射电子的颗粒辐射的绝对值。使用Monte Carlo辐射传输代码Penelope和Geant4进行了实验的模拟。测量和模拟结果的比较显示出良好的定性一致性。当模拟结果用曲线考虑考虑寿命扩展的效果时,光电子的线形状和与实验观察到的曲线相似。在绝对尺度上,实验倾向于在所研究的较低光子能量以及在Au L3光电子能量以下的电子能量的较高光子能量下以及在较高的光子能量下给出较高的电子辐射值。这归因于实验中光子束的线性极化,这在模拟代码中未考虑。
Electron emission spectra of a thin gold foil after photon interaction were measured over the energy range between 50 eV and 9500 eV to provide reference data for Monte Carlo radiation-transport simulations. Experiments were performed with the HAXPES spectrometer at the PETRA III high-brilliance beamline P22 at DESY (Hamburg, Germany) for photon energies just below and above each of the gold L-edges, i.e., at 11.9 keV, 12.0 keV, 13.7 keV, 13.8 keV, 14.3 keV, and 14.4 keV. The data were analyzed to obtain the absolute values of the particle radiance of the emitted electrons per incident photon flux. Simulations of the experiment were performed using the Monte Carlo radiation-transport codes Penelope and Geant4. Comparison of the measured and simulated results shows good qualitative agreement. When simulation results are convolved with curves that take into account the effect of lifetime broadening, line shapes of photoelectron and Auger peaks similar to those observed experimentally are obtained. On an absolute scale, the experiments tend to give higher electron radiance values at the lower photon energies studied as well as at the higher photon energies for electron energies below the energy of the Au L3 photoelectron. This is attributed to the linear polarization of the photon beam in the experiments which is not considered in the simulation codes.